The Puerto Rican rapper also brought conscious rap and funky energy to his set.
"I am thrilled to have been given the opportunity to go back and do it again as a full grown adult with my band and some newer songs," said Katie Crutchfield.
The dancehall legend heated up the NPR offices with a wide-ranging set of hits from his career.
The departure of Boilen, who also created and hosts All Songs Considered, follows news that two other high-level executives will soon exit the broadcaster.
"I'm Chloe -- Miss Bailey if you nasty."
The sibling trio are currently on their first-ever U.S. tour.
He reached back for mixtape song "seoul" and played a pair of tracks from his new "Indigo" solo album.